Raman scattering study of CS2 in CCI4
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چکیده
منابع مشابه
Polarized and magic angle fifth-order 2D elec- tronically non-resonant Raman scattering from CS2
We have successfully used phase matching considerations to provide significant discrimination against cascaded lower-order responses and measured the direct fifth-order response from the intermolecular motions in liquid CS2. Here we report the measured polarized and magic angle responses and discuss comparisons
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Actively phase-locked heterodyne-detected fifth-order nonresonant Raman scattering from room temperature CS2 has been measured. The experimental signals have similar magnitudes, shapes, and sign changes as calculated responses obtained via molecular dynamics simulations [S. Saito and I. Ohmine, Phys. Rev. Lett. 88, 207401 (2002)]. The measured signals contain sign changes that appear to be asso...
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In this paper we report the measurement of the direct fifth-order electronically nonresonant intermolecular response from liquid CS2 at room temperature. We recently demonstrated that all previous attempts to measure the direct fifth-order response were dominated by third-order cascaded signals @J. Chem Phys. 111, 3105 ~1999!#. Here we show that phase matching considerations can be used to prov...
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